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E-raamat: Advances In Multi-photon Processes And Spectroscopy, Vol 20

Edited by (Inst De Physique Et Chimie Des Materiaux De Strasbourg, France), Edited by (Tohoku Univ, Japan), Edited by (Nat'l Chiao-tung Univ, Taiwan, Inst Of Atomic & Molecular Sciences, Taiwan & Arizona State Univ, Usa)
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This book presents the latest developments and issues in both experimental and theoretical studies of multi-photon processes and the spectroscopy of atoms, molecules and nanomaterials in Physics, Chemistry, Biology and Material Science. It is an important addition to an advanced series that contains review papers suitable for both active researchers in these areas and non-experts who wish to enter the field. Special attention is paid to the recent progress of nonlinear photon-matter interactions applied to femtosecond laser induced nonadiabatic molecular alignment, high-order harmonic generation from C60 fullerene plasma, resonant femtosecond stimulated Raman spectroscopy and attosecond pulse generation, as well as near-field optical imaging of noble-metal nanoparticles and photoexcited ultrafast electron transfer in condensed phase.
1 Wave Packet Analysis of Femtosecond Stimulated Raman Spectroscopy
1(52)
K. Niu
B. Zhao
Z. Sun
Soo-Y. Lee
1 Introduction
2(1)
2 Theory
3(15)
2.1 Coupled wave theory of FSRS and its limitations
3(5)
2.2 Quantum theory of FSRS
8(10)
3 Applications, Results and Discussion
18(29)
3.1 Analytic results for FSRS from a stationary state with polyatomic harmonic potentials
18(6)
3.2 Application to FSRS of Rhodamine 6G
24(7)
3.3 Application to the FSRS from a coherent vibrational state of CDCl3
31(2)
3.3.1 Direct fifth-order process
33(3)
3.3.2 Cascade processes
36(5)
3.3.3 Direct fifth-order and cascade results of CDCl3
41(6)
4 Conclusion and outlook
47(6)
Acknowledgements
49(1)
References
49(4)
2 Field-Free Molecular Alignment by Two Femosecond Laser Pulses
53(48)
Chengyin Wu
Hongbing Jiang
Qihuang Gong
1 Introduction
53(2)
2 Theory
55(11)
2.1 Creation of rotational wavepacket
55(2)
2.2 Characterization of rotational wavepacket
57(3)
2.3 Control of rotational wavepacket
60(6)
3 Experimental Method
66(7)
4 Results and Discussion
73(14)
4.1 Manipulation of alignment structures
73(6)
4.2 Enhancement of molecular alignment
79(4)
4.3 Control of molecular population
83(4)
5 Applications of Field-Free Aligned Molecules --- Frequency Tuning of Few Cycle Femtosecond Laser Pulses
87(7)
5.1 Parameters
88(3)
5.2 Simulation
91(3)
6 Conclusions
94(7)
Acknowledgements
95(1)
References
95(6)
3 High-Order Harmonic Generation from C60 Fullerene Plasma
101(26)
T. Ozaki
1 Introduction
101(3)
2 Experimental Set-up
104(1)
3 Results and Discussion
105(18)
3.1 Observation of high-order harmonics from C60 fullerenes
105(3)
3.2 Influence of various experimental parameters on the HHG efficiency in fullerene plasma
108(7)
3.3 Simulations of harmonic spectra from C60 fullerenes
115(6)
3.4 Discussions
121(2)
4 Conclusions
123(4)
References
124(3)
4 Attosecond Pulse Generation, Characterization and Application
127(48)
Shouyuan Chen
Steve Gilbertson
He Wang
Michael Chini
Kun Zhao
Sabih Khan
Yi Wu
Zenghu Chang
1 Introduction
127(1)
2 Ultrafast Laser Development and CE Phase Stabilization for Attosecond Pulse Generation
128(9)
2.1 CE phase drift caused by the grating drift in stretcher and compressor
130(3)
2.2 CE phase stabilization of multi-pass and regenerative amplifiers
133(4)
3 Attosecond Gating Technology
137(9)
3.1 Two-color gating
139(1)
3.2 Polarization gating
140(2)
3.3 Double optical gating
142(1)
3.4 Generalized double optical gating
142(1)
3.5 DOG and GDOG optics
143(3)
4 Attosecond Pulse Measurement and Characterization
146(12)
4.1 Attosecond streak camera
146(5)
4.2 Frequency-resolved optical gating for complete reconstruction of attosecond bursts
151(3)
4.3 Phase retrieval by omega oscillation filtering
154(4)
5 Application of Attosecond Pulse
158(12)
5.1 Study of Helium autoionization by attosecond streaking
158(5)
5.2 Time resolved spectroscopy study of Argon
163(7)
6 Summary and Outlook
170(5)
References
170(5)
5 Near-Field Imaging of Optical-Field Structures and Plasmon Wave Functions in Metal Nanostructures
175(36)
Hiromi Okamoto
Kohei Imura
1 Introduction
175(2)
2 What can be Observed by Near-Field Optical Imaging?
177(11)
2.1 Near-field excitation of electromagnetic modes
177(2)
2.2 Analogy between the observation of electromagnetic modes and oscillating strings
179(2)
2.3 Electromagnetic modes and photonic local densities of states
181(3)
2.4 Optical transitions and wave functions of polarized excited states
184(3)
2.5 The eigenmodes of polarization waves on nanorods
187(1)
3 Basic Optical Characteristics of Gold Nanoparticles
188(2)
4 Experimental Methods of Near-Field Optical Microscopy
190(2)
5 Near-Field Optical Imaging of Noble-Metal Nanoparticles
192(8)
5.1 Near-field transmission spectra of spherical gold nanoparticles
192(2)
5.2 Near-field optical images of gold nanorods
194(3)
5.3 Near-field ultrafast pump-probe imaging of gold nanorod
197(2)
5.4 Near-field two-photon excitation images of gold nanorods
199(1)
6 Near-Field Optical Imaging of Noble Metal Nanoparticle Assemblies
200(4)
6.1 Localized optical field enhancement in spherical gold nanoparticle dimers
201(2)
6.2 Electric-field enhancements in many-particle assemblies
203(1)
7 Concluding Remarks
204(7)
Acknowledgements
205(1)
References
205(6)
6 Photoexcited Ultrafast Electron Transfer and Molecular Dynamics in Condensed Phase
211
Yutaka Nagasawa
Masayasu Muramatsu
1 Introduction
211(2)
2 Transition State Theory of Electron Transfer
213(1)
3 Multi-dimensional Reaction Coordinate
214(2)
4 Solvation Dynamics Measurement
216(8)
4.1 Dynamic stokes shift (DSS) measurement
216(3)
4.2 Three-pulse photon echo peak shift measurement (3PEPS)
219(5)
5 Ultrafast ET in Electron Donating Solvents
224(3)
6 Ultrafast ET in Ionic Liquids
227(5)
6.1 Solvation dynamics in ionic liquids
227(2)
6.2 Charge separation of 9,9'- bianthryl in ionic liquids
229(3)
7 Ultrafast LMCT Dynamics of Plastocyanin
232(10)
8 Conclusions
242
Acknowledgements
242(1)
References
242
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