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E-raamat: Advances In Multi-photon Processes And Spectroscopy, Volume 23

Edited by (Nat'l Chiao-tung Univ, Taiwan, Inst Of Atomic & Molecular Sciences, Taiwan & Arizona State Univ, Usa), Edited by (Inst De Physique Et Chimie Des Materiaux De Strasbourg, France), Edited by (Tohoku Univ, Japan)
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Advances In Multi-photon Processes And Spectroscopy, Volume 23Suurem pilt
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This volume presents recent progress and perspectives in multi-photon processes and spectroscopy of atoms, ions, and molecules. The subjects in the series cover the experimental and theoretical investigations in interdisciplinary research fields in natural science including chemistry, physics, bioscience and material science.
Preface v
1 Control of Radiationless Transitions
1(54)
Robert J. Gordon
Tamar Seideman
1 Introduction
1(2)
2 Adiabatic and Diabatic Transitions
3(9)
2.1 Breakdown of the BO approximation
3(3)
2.2 Conical intersections and seams
6(6)
3 Environmental Control
12(2)
4 Optical Control in Weak Fields
14(12)
4.1 Overview
14(1)
4.2 Eigenstate control
15(4)
4.3 Weak field coherent control of radiationless transitions
19(4)
4.4 Coherent control via overlapping resonances
23(3)
5 Optical Control at Intermediate Field Strengths
26(6)
6 Optical Control in Strong Fields
32(9)
7 Coherent versus Incoherent Control in Liquids
41(4)
8 Summary and Outlook
45(10)
Acknowledgments
49(1)
References
49(6)
2 Optimal Control Approaches for Aligning/Orienting Linear Molecules
55(42)
Yukiyoshi Ohtsuki
Masataka Yoshida
Kaoru Nakashima
Kenta Arai
Katsuhiro Nakajima
1 Introduction
55(7)
1.1 Field-free molecular alignment control
58(1)
1.2 Field-free molecular orientation control
59(3)
2 Optimal Control Simulation with Nonlinear Interactions
62(14)
2.1 Hamiltonian
63(1)
2.2 Optimal control simulation in wave function formalism
64(3)
2.3 Inclusion of polarization effects
67(2)
2.4 Introducing instantaneous penalty
69(1)
2.5 Optimal control simulation in finite-temperature cases (density operator formalism)
70(3)
2.6 Two-color excitation schemes for molecular orientation control
73(1)
2.6.1 Phase-locked two-color laser pulse
74(1)
2.6.2 Combination of THz and laser pulses
75(1)
3 Numerical Examples
76(13)
3.1 Alignment control in the low-temperature limit
76(4)
3.2 Orientation control by using phase-locked two-color laser pulses
80(4)
3.3 Orientation control with a combination of THz and laser pulses at finite temperature
84(5)
4 Outlook
89(1)
5 Summary
90(7)
Acknowledgments
91(1)
References
91(6)
3 Femtosecond Laser-Induced Coulomb Explosion Imaging
97(58)
Reza Karimi
Wing-Ki Liu
Joseph Sanderson
1 Introduction
97(3)
2 Strong Field Ionization and Laser Assisted Coulomb Explosion
100(5)
2.1 Theoretical considerations
100(2)
2.2 Recent experimental studies
102(3)
3 Experimental Set-up
105(11)
3.1 The laser system
105(1)
3.2 Time of flight (TOF) spectrometer
106(2)
3.3 Data reduction and coincidence identification
108(1)
3.3.1 General analysis technique
109(1)
3.3.2 Coincidence technique
110(2)
3.3.3 Efficiency
112(2)
3.3.4 Momentum filtering in coincidence identification
114(2)
4 Ionization and Dissociation Dynamics of CO2
116(15)
4.1 Coulomb explosion of CO2
117(1)
4.2 TOF spectra
118(5)
4.3 Molecular structure reconstruction and theoretical calculations
123(4)
4.4 Dalitz and Newton plots
127(4)
5 Ionization and Dissociation Dynamics of N2O and OCS
131(17)
5.1 N2O under femtosecond laser radiation
131(1)
5.1.1 TOF spectra
132(1)
5.1.2 Dalitz plots
133(4)
5.1.3 Kinetic energy release
137(3)
5.2 Ionization and dissociation dynamics of OCS
140(5)
5.2.1 Imaging control of dissociation processes using FEMPULS
145(3)
6 Conclusions and Future Prospects
148(7)
Acknowledgments
148(1)
References
149(6)
4 Development of Ultrashort Pulse Lasers and their Applications to Ultrafast Spectroscopy in the Visible and NIR Ranges
155(56)
Takayoshi Kobayashi
1 Generation of 5-fs Visible Pulses form a Non-collinear Optical Parametric Amplifier
156(23)
1.1 Basics of ultrashort pulse generation by a non-collinear parametric amplifier
156(1)
1.1.1 Nonlinear optical processes and nonlinear susceptibilities
156(2)
1.1.2 OPA
158(4)
1.2 Broad band condition for phase-matching in type-I BBO crystal
162(3)
1.3 Type-I phase-matching condition in BBO crystal
165(3)
1.4 Optical parametric fluorescence
168(1)
1.5 Parametric gain spectrum
169(2)
1.6 Pulse front tilting
171(4)
1.7 Experimental setup
175(1)
1.7.1 NOPA setup
175(2)
1.7.2 Pump-probe experimental setup
177(2)
2 Spectral Oscillation Observed in Optical Frequency Resolved Quantum-beat Spectroscopy with a 6-fs Laser
179(17)
2.1 Introduction basics of quantum beat spectroscopy
179(1)
2.1.1 Quantum-beat spectroscopy
179(2)
2.1.2 Vibrational quantum beat spectroscopy
181(3)
2.1.3 Amplitudes and phases of optical field and molecular vibration
184(2)
2.1.4 Principal of real-time vibrational spectroscopy
186(3)
2.2 Experiment
189(1)
2.2.1 Material
189(1)
2.2.2 Ultrashort pulse laser system
190(1)
2.3 Coupling of optical field with coherent vibrational modes in molecules
191(1)
2.3.1 A-type and V-type interactions
191(2)
2.3.2 Coherent molecular vibration modes interaction with ultrashort pulses
193(1)
2.3.3 Pumping process
194(1)
2.3.4 Probing process
195(1)
3 Results and Discussion
196(6)
3.1 Experimental results
196(1)
3.1.1 Real-time traces
196(1)
3.1.2 2D difference absorption spectrum and the Fourier power spectrum
197(1)
3.2 Analysis and discussion
198(1)
3.2.1 Probe photon energy dependence of the Fourier power
198(2)
3.2.2 Origins of the Fourier power spectrum depending on the probe photon energy
200(2)
4 Conclusion
202(9)
Acknowledgments
204(1)
References
204(7)
5 Nonlinear Optical Properties in Molecular Systems with Non-Zero Permanent Dipole Moments in Four-Wave Mixing under Stochastic Considerations
211(38)
J. L. Paz
A. Mastrodomenico
Jaime F. Cardenas-Garcia
Luis G. Rodriguez
Cesar Costa Vera
1 Introduction
212(1)
2 Theoretical Considerations
213(2)
3 Stochastic Description
215(1)
4 Perturbative Treatment
216(6)
5 Average of the Events
222(3)
6 Nonlinear Macroscopic Polarization
225(9)
7 Results and Discussion
234(15)
7.1 Final comments
244(3)
Acknowledgments
247(1)
References
247(2)
Index 249
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