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E-raamat: Biosphere Implications Of Deep Disposal Of Nuclear Waste: The Upwards Migration Of Radionuclides In Vegetated Soils

(Imperial College London, Uk & Univ Of Nottingham, Uk), (Imperial College London, Uk), (Imperial College London, Uk), (Imperial College London, Uk & Us Salinity Lab, Riverside, California, Usa), (Univ Of Saskatchewan, Canada)
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The safety assessment of a deep repository for nuclear waste poses challenging scientific and technical questions. The risks from leakage of radionuclides from the repository, including transfers to the biosphere and the food chain must be assessed. This involves complex and poorly understood interactions between groundwater, soils, plants and the atmosphere. A unique, multidisciplinary experimental and modeling program at Imperial College London has been funded by UK NIREX to develop the science and to produce modeling tools to interpret and generalize the experimental data for safety assessment. This monograph brings together for the first time the accumulated results and experience from almost two decades of research. The results have important implications for the safety assessment of nuclear waste worldwide and provide new insights into the geochemical and biological controls on the upwards migration of radiochemicals in the near-surface environment.
Acknowledgements v
Preface vii
Section 1 Background
1(10)
Introduction
3(8)
Section 2 Methods
11(76)
Experimental Protocols
13(28)
Background
13(1)
Phase I and II Lysimeter Experiments
14(15)
Soil Column Experiments
29(6)
Mini-column Experiments
35(6)
Modelling Radionuclide Transport and Uptake in Vegetated Soils
41(46)
Introduction
41(1)
Lysimeter System Model
42(15)
Physically-Based Modelling
57(7)
Hydrological Model Applications
64(20)
Discussion
84(3)
Section 3 Results
87(256)
Radiochlorine
89(99)
Background
89(1)
Experimental Overview
90(3)
Results
93(91)
General Discussion
184(4)
Radioiodine
188(42)
Background
188(4)
Experimental Overview
192(2)
Results
194(32)
General Discussion
226(4)
Technetium
230(36)
Background
230(7)
Experimental Overview
237(1)
Results
238(25)
General Discussion
263(3)
Radioselenium
266(34)
Background
266(3)
Experimental Overview
269(1)
Results
269(25)
General Discussion
294(6)
Radiocations
300(43)
Background
300(1)
Experimental Overview
301(4)
Results
305(33)
General Discussion
338(5)
Section 4 Conclusions and Recommendations
343(24)
Conclusions
345(22)
Overview
345(1)
Summary of Results
346(15)
Experimental Design
361(2)
Modelling
363(2)
Conclusions and Future Directions
365(2)
Colour Section 367(12)
Appendix 379(2)
Data Archive 381(2)
Reference 383(14)
Index 397