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E-raamat: Catalytic Activation and Functionalisation of Light Alkanes: Advances and Challenges

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Catalytic Activation and Functionalisation of Light Alkanes: Advances and ChallengesSuurem pilt
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Because of C 1-C 4 alkanes relative stability of C-C and C-H bonds, they cannot yet be easily substituted for more expensive alkanes and aromatics in the catalysis processes of the petroleum, petrochemicals, and bulk and fine chemicals industries. The key issues in these 26 papers, then, is how to identify and achieve novel catalytic mechanisms by which light alkanes can be activated in mild conditions, functionalized, and reacted selectively, while ensuring satisfactory catalyst stability and life. Containing all the lectures and selected communications from an ASI conference bearing the same title as this book (held in Portugal, May/June, 1997), the material encompasses topics which range from homogeneous to heterogeneous approaches, and highly theoretical and experimental methods. Annotation c. by Book News, Inc., Portland, Or.

Light alkanes tend to be resistant to many forms of activation. The horizontal approach of the present book covers homogeneous, heterogeneous and biological catalysis, thus allowing readers to gain an awareness of progress and ideas in research areas different from their own. The book contains both general chapters, giving an overview of the subject, and specialised contributions that deal with the details and state of the art. A specialist report is also included which gives a critical insight into current progress and discusses future prospects and major challenges. Audience: Newcomers and senior researchers in the field of alkane activation. The mixed theoretical and practical approach will be of interest to researchers and industrialists alike.

Arvustused

`... an important contribution towards the integration of different approaches to catalysis, as advocated in the Workshop report, and is sure to find its way on to the shelves of many laboratories in which catalysis research is being pursued or considered.' Applied Organometallic Chemistry, 13 (1999)

Preface ix SECTION 1 - LECTURES 1(388) Upgrading of C1 and C2 Hydrocarbons 3(32) P.L. Villa S. Rapagna Transformation of Alkanes on Solid Acid and Bifunctional Catalysts 35(40) Avelino Corma Agustin Martinez Activation of Light Alkanes: Past and Present 75(14) Ivan V. Kozhevnikov Superacid Catalysed Protolytic Activation, H/D Exchange and Oxidation of Small Alkanes 89(22) J. Sommer J. Bukala M. Hachoumy R. Jost New Processes for Carbon-Carbon Bond Activation Catalysed by Oxyde Supported Surface Organometallic Complexes 111(14) Gerald P. Niccolai Jean-Marie Basset Selective Oxidation of Light Alkanes 125(32) G.J. Hutchings Theoretical Basis of the Activation of C-H Bond 157(32) Jerzy Haber An Introduction to Molecular Heterogeneous Catalysis 189(26) C.R.A. Catlow R.G. Bell J.D. Gale D.W. Lewis D.C. Sayle P.E. Sinclair Mono- and Binuclear Iron Complexes in Zeolites and Mesoporous Oxides as Biomimetic Alkan Oxidation Catalysts 215(44) P.P. Knops-Gerrits A.-M. Van Bavel G. Langouche P.S. Jacobs Biocatalytic, Biomimetic and Suprabiotic Oxidation of Alkanes 259(38) R.A. Sheldon High Yield, Low Temperature Oxidation of Methane to Methanol 297(14) Roy A. Periana Douglas J. Taube Scott Gamble Henry Taube Hiroshi Fuji Functionalization of Light Alkanes Catalyzed by Heteropoly Compounds 311(22) Noritaka Mizuno Makoto Misono Alkane Activation by Pseudo-Metals 333(36) G. Djega-Mariadassou Molecular Chemistry of Alkane Activation: Formation and Reaction of Chx Species on Metal Surfaces 369(20) F. Solymosi SECTION 2 - COMMUNICATIONS 389(64) The Effect of Acid Sites in Skeletal Isomerization of n-Butenes over Ferrierites and CoAlPO-11 391(6) Jiri Cejka Nadezda Zilkova Zdena Tvarozova Blanka Wichterlova Oxidative Dehydrogenation of Propane on Large-Pore Zeolites 397(6) Miroslaw Derewinski Joanna Krysciak Zbigniew Olejniczak Bogdan Sulikowski Gema Bueno Vicente Cortes Corberan Rita Ximena Valenzuela Oxidative Coupling of Methane over Sodium-Manganese Catalysts in the Presence of HCl 403(10) E.V. Shischak M.S. Kazi I.P. Dzikh S.S. Abadjev V.U. Shevchuk Mono- and Binuclear Iron Complexes in Zeolites, Clays and Mesoporous Oxides as Biomimetic Catalysts 413(4) P.P. Knops-Gerrits P.A. Jacobs Mixed M2O3.Zro2.SO42- (M = Ga, In, Tl) Catalysts: Preparation, Characterisation and Catalytic Behaviour in Dehyroisomerisation of n-Hexane 417(6) V. Parvulescu S. Coman P. Grange V.I. Parvulescu The Selective Oxidation of n-Butane to Maleic Anhydride; Development of Silica- and Titania Supported V-P-O Catalysts 423(6) Matthijs Ruitenbeek R.A. Overbeek D.C. Koningsberger J.W. Geus The Effect of Cobalt Doping on the Structural Transformation Sequences Occurring during the Activation of Vanadium Phosphorus Oxide Catalysts 429(6) S. Sajip C. Rhodes J.K. Bartley A. Burrows C.J. Kiely C.J. Hutchings On the Active Sites for Selective Ammoxidation of Propane on Vanadium Containing Oxide Catalysts 435(4) Horst Zanthoff Theoretical Modelling of Propane Partial Oxidation over Titanium Silicalites 439(8) Georgi N. Vayssilov Chlorinated Alumina Catalyst for Isobutane / 2-Butene Alkylation: Influence of Added Noble Metals 447(6) J.M. Goupil G. Clet F. Hemming-Maire D. Cornet G. Szabo P. Nascimento R. Loutaty SECTION 3 - EC WORKSHOP 453(14) Report of the Workshop on Challenges and Opportunities in Light Alkane Activation 455(12) Jay A. Labinger Graham J. Hutchings List of Participants 467(16) Subject Index 483(6) Author Index 489
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